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Multifunctional far-field luminescence nanoscope for studying single molecules and quantum dots

 a, b,  a, b, c,  a, d, b
a Moscow Institute of Physics and Technology (National Research University), Institutskii per. 9, Dolgoprudny, Moscow Region, 141701, Russian Federation
b Institute of Spectroscopy, Russian Academy of Sciences, ul. Fizicheskaya 5, Troitsk, Moscow, 108840, Russian Federation
c École Polytechnique Fédérale de Lausanne, Lausanne, Switzerland
d Moscow State Pedagogical University, M. Pirogovskay, 1, Moscow, 119435, Russian Federation

Far-field fluorescence spectromicroscopy of single quantum emitters (SQE) (organic molecules, quantum dots, color centers in crystals) is one of the actively developing fields of modern photonics, which is widely demanded in various applications in physics, chemistry, material sciences, life sciences, quantum technologies. In this paper we present a description of multifunctional experimental setup, which was developed last years in the Institute for Spectroscopy of the Russian Academy of Sciences. It allows to measure optical spectra and fluorescence images of SQE, as well as their temporal behavior and luminescence kinetics, in a broad range of temperatures (from cryogenic to ambient). It is shown that spatial coordinates of SQE can be reconstructed with subdiffractional accuracy (up to a few Angstroms). Some examples of the developed methods for multiparameter superresolution microscopy (nanoscopy) of materials and nanostructures are presented.

Fulltext pdf (777 KB)
Fulltext is also available at DOI: 10.3367/UFNe.2018.06.038461
Keywords: luminescence, microscopy, nanoscopy, single molecule, quantum dot, color center, antibunching, kinetics, polymers, glasses, crystals, nanodiagnostics, cryogenic temperatures, Shpol'skii matrix, sensor, CdSe, NV-center
PACS: 42.79.−e, 78.55.−m, 78.67.Hc (all)
DOI: 10.3367/UFNe.2018.06.038461
URL: https://ufn.ru/en/articles/2019/3/i/
000469214700009
2-s2.0-85069480377
2017DokPh..62..294N
Citation: Eremchev I Yu, Eremchev M Yu, Naumov A V "Multifunctional far-field luminescence nanoscope for studying single molecules and quantum dots" Phys. Usp. 62 294–303 (2019)
BibTexBibNote ® (generic)BibNote ® (RIS)MedlineRefWorks

Received: 28th, August 2018, 20th, June 2018

Оригинал: Еремчев И Ю, Еремчев М Ю, Наумов А В «Многофункциональный люминесцентный наноскоп дальнего поля для исследования одиночных молекул и квантовых точек (к 50-летию Института спектроскопии РАН)» УФН 189 312–322 (2019); DOI: 10.3367/UFNr.2018.06.038461

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