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Превращение беспорядок–порядок и фазовые равновесия в сильно нестехиометрических соединениях


Институт химии твердого тела УрО РАН, ул. Первомайская 91, Екатеринбург, 620219, Российская Федерация

Обобщены результаты исследований фазовых превращений беспорядок–порядок, происходящих в сильно нестехиометрических карбидах и нитридах MXy (X = C, N) переходных металлов IV и V групп при температуре ниже 1300–1400 K. Обсуждено применение метода функционала параметров порядка для описания атомно-вакансионного упорядочения сильно нестехиометрических соединений MXy и расчета фазовых равновесий в системах M–X. Приведены фазовые диаграммы систем Ti–C, Zr–C, Hf–C, Nb–C, Ta–C, V–C, Ti–N, Ti–B–C, построенные с учетом упорядочения нестехиометрических карбидов и нитридов, а также фазовые диаграммы псевдобинарных карбидных систем M(1)C–M(2)C. Рассмотрено изменение теплоемкости, электросопротивления, магнитной восприимчивости нестехиометрических карбидов при обратимых переходах порядок–беспорядок.

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English fulltext is available at DOI: 10.1070/PU2000v043n01ABEH000647
PACS: 61.72.Ji, 64.60.Cn, 81.30.Dz (все)
DOI: 10.3367/UFNr.0170.200001a.0003
URL: https://ufn.ru/ru/articles/2000/1/a/
000086055100001
Цитата: Гусев А И "Превращение беспорядок–порядок и фазовые равновесия в сильно нестехиометрических соединениях" УФН 170 3–40 (2000)
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English citation: Gusev A I “Order-disorder transformations and phase equilibria in strongly nonstoichiometric compounds” Phys. Usp. 43 1–37 (2000); DOI: 10.1070/PU2000v043n01ABEH000647

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