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Фуллерены в растворах

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Национальный исследовательский центр «Курчатовский институт», пл. акад. Курчатова 1, Москва, 123182, Российская Федерация

Рассмотрены явления и процессы, связанные с поведением фуллеренов в растворах. Представлены имеющиеся данные о растворимости фуллеренов С60 и C70 в большом числе растворителей при различных температурах, а также о коэффициенте диффузии фуллеренов в растворах. Проанализирована связь явлений, определяющих поведение фуллеренов в растворах, с тенденцией фуллеренов в растворах к образованию кластеров, состоящих из некоторого количества молекул. Эта тенденция, отличающая фуллерены от других крупных молекул, приводит к таким особенностям в поведении фуллеренов в растворах, как обнаруженная недавно немонотонная температурная зависимость растворимости фуллеренов в различных растворителях, нелинейная концентрационная зависимость нелинейной оптической восприимчивости, резкая зависимость окраски раствора фуллерена от состава растворителя (сольватохроматический эффект), концентрационная зависимость теплоты растворимости фуллеренов в органических растворителях и т.п. Проанализированы механизмы роста фрактальных кластеров в растворах фуллеренов, а также законы подобия, определяющие термодинамические характеристики кристаллов фуллеритов.

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English fulltext is available at DOI: 10.1070/PU1998v041n11ABEH000502
PACS: 36.40.−c, 61.46.+w, 61.48.+c (все)
DOI: 10.3367/UFNr.0168.199811b.1195
URL: https://ufn.ru/ru/articles/1998/11/b/
000077738800002
Цитата: Безмельницын В Н, Елецкий А В, Окунь М В "Фуллерены в растворах" УФН 168 1195–1220 (1998)
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English citation: Bezmel’nitsyn V N, Eletskii A V, Okun’ M V “Fullerenes in solutions” Phys. Usp. 41 1091–1114 (1998); DOI: 10.1070/PU1998v041n11ABEH000502

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