RSS feeds
РусскийEnglish
Issue 9, 2026
Volume year page
Issues Authors PACS Subscription For authors

Issues

 / 

2019

 / 

March

←  →

From the current literature


On a half-forgotten but very powerful method for coherent spectroscopy of molecules

 a, b,  a
a Institute of Spectroscopy, Russian Academy of Sciences, ul. Fizicheskaya 5, Troitsk, Moscow, 108840, Russian Federation
b HSE University, ul. Myasnitskaya 20, Moscow, 101000, Russian Federation

The sum-frequency generation involving two infrared laser quanta and a single visible-range laser quantum is a four-wave mixing process that is virtually not used in practice. Nevertheless, this process provides an extremely high selectivity with respect to the Q-branch of the two-photon vibrational transition in molecules. We explore here two publications, one that is more than thirty years old and another that appeared in 2018, to show broad potential applications of the method. The objective reasons due to which that potential has not been used so far are discussed.

Fulltext pdf (557 KB)
Fulltext is also available at DOI: 10.3367/UFNe.2018.12.038492
Keywords: sum frequency generation, two-photon resonance, infrared spectroscopy of molecules
PACS: 33.20.Ea, 42.62.Fi, 42.65.−k (all)
DOI: 10.3367/UFNe.2018.12.038492
URL: https://ufn.ru/en/articles/2019/3/c/
000469214700003
2-s2.0-85069429219
2019PhyU...62..257M
Citation: Makarov A A, Ryabov E A "On a half-forgotten but very powerful method for coherent spectroscopy of molecules" Phys. Usp. 62 257–265 (2019)
BibTexBibNote ® (generic)BibNote ® (RIS)MedlineRefWorks

Received: 11th, July 2018, revised: 5th, December 2018, 6th, December 2018

Оригинал: Макаров А А, Рябов Е А «Об одном полузабытом, но весьма мощном методе когерентной спектроскопии молекул» УФН 189 271–280 (2019); DOI: 10.3367/UFNr.2018.12.038492

References (57) ↓ Cited by (2) Similar articles (20)

  1. Traverso A J et al Phys. Rev. Lett. 120 063602 (2018)
  2. ’Bkh’?’?’?’?’? ’l ’B, ’F’?р’?т’?’?’? ’v ’R Usp. Fiz. Nauk 123 405 (1977); Akhmanov S A, Koroteev N I Sov. Phys. Usp. 20 899 (1977)
  3. ’Bkh’?’?’?’?’? ’l ’B, ’F’?р’?т’?’?’? ’v ’R ’a’?т’?’?ы ’?’?’?’?’?’?’?’?’?’? ’?’?т’?’?’? ’? с’?’?’?тр’?с’?’?’?’?’? р’?сс’?ya’?’?ya с’?’?т’? (’a.: ’v’?у’?’?, 1981)
  4. Akhmanov S A Nonlinear Spectroscopy (Ed. N Bloembergen) (Amsterdam: North Holland, 1977), Ch. 9; ’z’?р. ’?’? русс’?. ya’?., ’Bkh’?’?’?’?’? ’l ’B ’v’?’?’?’?’?’?’?’?ya с’?’?’?тр’?с’?’?’?’?ya (’z’?’? р’?’?. ’v ’G’?’?’?’?’?р’?’?’?’?) (’a.: ’a’?р, 1979) с. 267
  5. Kildal H, Brueck S R J Phys. Rev. Lett. 38 347 (1977)
  6. Kung R T V, Many S A Appl. Phys. 50 2548 (1979)
  7. ’Bkh’?’?’?’?’? ’l ’B ’? ’?р ’z’?сь’?’? Zh’n’s 5 1507 (1979)
  8. Chung K M, Stevens G, Becker M F IEEE J. Quantum Electron. 15 874 (1979)
  9. ’M’?с’?’?’? ’R ’E, ’iу’?ts’?’?’? ’v ’v, ’l’?’?’?рts’?’? ’E ’E ’F’?’?’?р’?’?т’?ы’? ’?’?р’?kh’?’?’?ы’? ’?р’?ts’?ссы ’? ’?’?т’?’?’? (’a.: ’s’?’?’?’?т’?’?т, 2009), ’I’?. 2
  10. ’O’?’?ь’?’?’?’?ch ’G Ya, ’z’?’?’?’?’?ts’?’?’? ’v ’s, Sh’?у’?’?’? ’E ’E Usp. Fiz. Nauk 138 249 (1982); Zel’dovich B Ya, Pilipetskii N F, Shkunov V V Sov. Phys. Usp. 25 713 (1982)
  11. ’’’?т’?kh’?’? ’E ’l, Ch’?’?’?т’?’?’? ’E ’z ’v’?’?’?’?’?’?’?’?ya ’?’?’?’?р’?’?ya с’?’?’?тр’?с’?’?’?’?ya с’?’?рkh’?ыс’?’?’?’?’? р’?’?р’?sh’?’?’?ya (’a.: ’v’?у’?’?, 1990), ’I’?. 6
  12. ’K’?’?zh’?’?’?’? ’E ’l ’? ’?р Kvantovaya Elektron. 13 887 (1986); Dolzhikov V S et al Sov. J. Quantum Electron. 16 580 (1986)
  13. Pellin M J, Yardley J T Appl. Phys. Lett. 29 304 (1976)
  14. ’Bkh’?’?’?’?’? ’l ’B ’F’?’?’?т’?’?’?ya э’?’?’?тр’?’?. 3 1846 (1976); Akhmanov S A Sov. J. Quantum Electron. 6 1012 (1976)
  15. ’E’?р’?’?’?’? ’E ’v, ’I’?р’?’?’?’?’?’? ’E ’a, ’’’?’?’?т’?’? ’B ’s ’zр’?’?р’?’?т №3 (’a.: ’s’?’?’?ch’?с’?’?’? ф’?’?у’?ьт’?т ’a’I’p, 1981)
  16. ’E’?р’?’?’?’? ’E ’v, ’I’?р’?’?’?’?’?’? ’E ’a ’nру’?ы VII ’E’?’?’?’?’?’?с’?’?’? ’?’?’?ф’?р’?’?ts’?’? ’?’? ’?’?’?’?’?’?’?’?’?’? ’?’?т’?’?’?, ’?yu’?ь 1981 ’?. Т. 2 (’z’?’? р’?’?. ’l ’I ’i’?ут’?’?’?’?) (’v’?’?’?с’?’?’?рс’?: ’R’?ст’?тут ’?’?т’?’?’?т’?’?’? ’? э’?’?’?тр’?’?’?тр’?’? ’l’d ’B’v ’l’l’l’i, 1982) с. 214
  17. Zh’?’?т’?’?’?’? ’B ’a, ’F’?р’?т’?’?’? ’v ’R Usp. Fiz. Nauk 169 385 (1999); Zheltikov A M, Koroteev N I Phys. Usp. 42 321 (1999)
  18. di Lauro C, Mills I M J. Mol. Spectrosc. 21 386 (1966)
  19. Smith A L Applied Infrared Spectroscopy (1979); ’z’?р. ’?’? русс’?. ya’?., ’l’?’?т ’B ’zр’?’?’?’?’?’?’?ya ’R’F-с’?’?’?тр’?с’?’?’?’?ya: ’?с’?’?’?ы, т’?kh’?’?’?’?, ’?’?’?’?’?т’?ch’?с’?’?’? ’?р’?’?’?’?’?’?’?’? (’a.: ’a’?р, 1982)
  20. Bürger H, Burczyk K, Schulz P Spectrochim. Acta A 38 627 (1982)
  21. ’O’?с’?’?’?с’?’?’? ’I ’a, Ch’?р’?’?’?’? ’G ’E Usp. Fiz. Nauk 105 3 (1971); Zaslavskii G M, Chirikov B V Sov. Phys. Usp. 14 549 (1972)
  22. ’I’?’?’?’?’?’?-’Iр’?kh’?’? ’B ’E, ’i’?’?’?’?’?’?’?ch ’a ’R Usp. Fiz. Nauk 128 579 (1979); Gaponov-Grekhov A V, Rabinovich M I Sov. Phys. Usp. 22 590 (1979)
  23. Chirikov B V Phys. Rep. 52 265 (1979)
  24. Lichtenberg A J, Liberman M A Regular And Stochastic Motion (New York: Springer, 1983); ’z’?р. ’?’? русс’?. ya’?., ’’’?khт’?’?’?’?р’? ’B, ’’’?’?’?р’?’?’? ’a ’i’?’?у’?yaр’?’?ya ’? ст’?kh’?ст’?ch’?с’?’?ya ’?’?’?’?’?’?’?’? (’a.: ’a’?р, 1984)
  25. ’O’?с’?’?’?с’?’?’? ’I ’a ’lт’?kh’?ст’?ch’?’?сть ’?’?’?’?’?’?ch’?с’?’?kh с’?ст’?’? (’a.: ’v’?у’?’?, 1984); ’z’?р. ’?’? ’?’?’?’?. ya’?., Zaslavsky G M Chaos In Dynamic Systems (New York: Harwood Acad. Publ., 1985)
  26. Gutzwiller M C Chaos In Classical And Quantum Mechanics (New York: Springer, 1990)
  27. Ott E Chaos In Dynamical Systems (New York: Cambridge Univ. Press, 1993)
  28. Lehmann K K, Scoles G, Pate B H Annu. Rev. Phys. Chem. 45 241 (1994)
  29. Nesbitt D J, Field R W J. Phys. Chem. 100 12735 (1996)
  30. ’a’?’?’?р’?’? ’B ’B, ’a’?’?’?’?’?’?с’?’?’? ’B ’’, ’iya’?’?’? ’M ’B Usp. Fiz. Nauk 182 1047 (2012); Makarov A A, Malinovsky A L, Ryabov E A Phys. Usp. 55 977 (2012)
  31. Doljikov Yu S et al Chem. Phys. Lett. 124 304 (1986)
  32. ’K’?’?zh’?’?’?’? Yu ’l ’? ’?р Zh. Eksp. Teor. Fiz. 90 1982 (1986); Dolzhikov Yu S et al Sov. Phys. JETP 63 1161 (1986)
  33. Yamada Y et al J. Chem. Phys. 120 7400 (2004)
  34. Chekalin S V et al J. Phys. Chem. A 118 955 (2014)
  35. Yoo H S, DeWitt M J, Pate B H J. Phys. Chem. A 108 1348 (2004)
  36. ’a’?’?’?’?’?’?с’?’?’? ’B ’’, ’a’?’?’?р’?’? ’B ’B, ’iya’?’?’? ’M ’B ’z’?сь’?’? Zh’e’n’s 80 605 (2004); Malinovsky A L, Makarov A A, Ryabov E A JETP Lett. 80 532 (2004)
  37. Malinovsky A L et al Chem. Phys. Lett. 419 511 (2006)
  38. ’a’?’?’?’?’?’?с’?’?’? ’B ’’, ’a’?’?’?р’?’? ’B ’B, ’iya’?’?’? ’M ’B Zh. Eksp. Teor. Fiz. 133 45 (2006); Malinovsky A L, Makarov A A, Ryabov E A JETP 106 34 (2006)
  39. Makarov A A, Malinovsky A L, Ryabov E A J. Chem. Phys. 129 116102 (2008)
  40. Malinovsky A L, Makarov A A, Ryabov E A ’z’?сь’?’? Zh’e’n’s 93 139 (2011); Malinovsky A L, Makarov A A, Ryabov E A JETP Lett. 93 124 (2011)
  41. Ebata T et al J. Phys. Chem. A 105 8623 (2001)
  42. Yamada Y, Mikami N, Ebata T J. Chem. Phys. 121 11530 (2004)
  43. Yamada Y et al J. Chem. Phys. 123 124316 (2005)
  44. Myers D J et al Chem. Phys. Lett. 312 399 (1999)
  45. Stromberg C, Myers D J, Fayer M D J. Chem. Phys. 116 3540 (2002)
  46. ’F’?’?’?’?’?’?ts ’E ’d ’? ’?р ’z’?сь’?’? Zh’e’n’s 92 157 (2010); Kompanets V O et al JETP Lett. 92 135 (2010)
  47. Chekalin S V et al Chem. Phys. Lett. 512 178 (2011)
  48. ’’’?’?’?’?у ’’ ’K, ’’’?фsh’?ts ’M ’a ’F’?’?’?т’?’?’?ya ’?’?kh’?’?’?’?’?. ’v’?р’?’?yaт’?’?’?стс’?’?ya т’?’?р’?ya (’a.: ’s’?’?’?’?т’?’?т, 1963) с. 440; ’z’?р. ’?’? ’?’?’?’?. ya’?., Landau L D, Lifshitz E M Quantum Mechanics: Non-Relativistic Theory (Oxford: Pergamon Press, 1965)
  49. Gustafson E K, McDaniel J C, Byer L R Opt. Lett. 7 434 (1982)
  50. Born M, Oppenheimer R Ann. Physik 84 457 (1927)
  51. Page R H, Shen Y R, Lee Y T Phys. Rev. Lett. 59 1293 (1987)
  52. Page R H, Shen Y R, Lee Y T J. Chem. Phys. 88 4621 (1988)
  53. Bagratashvili V N et al Opt. Commun. 9 135 (1973)
  54. ’G’?’?р’?т’?sh’?’?’?’? ’E ’v, ’F’?ya’?’?’? ’R ’v, ’’’?’?’?’? ’E ’E Kvantovaya Elektron. 2 1577 (1975); Bagratashvili V N, Knyazev I N, Lobko V V Sov. J. Quantum Electron. 5 857 (1975)
  55. ’G’?’?р’?т’?sh’?’?’?’? ’E ’v ’? ’?р Kvantovaya Elektron. 3 1011 (1976); Bagratashvili V N et al Sov. J. Quantum Electron. 6 541 (1976)
  56. Vitiello S M et al Opt. Express 23 5167 (2015)
  57. ’a’?тр’?ф’?’?’?’? ’B ’E ’? ’?р Usp. Fiz. Nauk 185 97 (2015); Mitrofanov A V et al Phys. Usp. 58 89 (2015)
© 1918–2026 Uspekhi Fizicheskikh Nauk
Email: ufn@ufn.ru Editorial office contacts About the journal Terms and conditions