RSS feeds
РусскийEnglish
Issue 12, 2024
Volume year page
Issues Authors PACS Subscription For authors

Issues

 / 

2006

 / 

January

←  →



Blinking fluorescence of single molecules and semiconductor nanocrystals


Lebedev Physical Institute, Russian Academy of Sciences, Leninsky prosp. 53, Moscow, 119991, Russian Federation

Papers are discussed in which the quantum dynamics of individual molecules and semiconductor nanocrystals is studied from their fluctuating fluorescence. Presented are the fundamental tenets of the theory of photon emission by a single nanoparticle irradiated by continuous laser light. Fluorescence fluctuations which occur only for single nanoparticles are shown to open up entirely new opportunities for investigating nanoparticle quantum dynamics. It is shown how the theory can be harnessed to analyze the fluorescence fluctuations of an individual polymer molecule and a semiconductor nanocrystal and how the corresponding microscopic models can be constructed proceeding from this analysis.

Fulltext pdf (460 KB)
Fulltext is also available at DOI: 10.1070/PU2006v049n01ABEH002088
PACS: 33.50.−j, 33.70.−w, 78.67.−n (all)
DOI: 10.1070/PU2006v049n01ABEH002088
URL: https://ufn.ru/en/articles/2006/1/b/
000237789100002
2-s2.0-33744499245
2006PhyU...49...19O
Citation: Osad’ko I S "Blinking fluorescence of single molecules and semiconductor nanocrystals" Phys. Usp. 49 19–51 (2006)
BibTexBibNote ® (generic)BibNote ® (RIS)MedlineRefWorks

Оригинал: Осадько И С «Флуктуирующая флуоресценция одиночных молекул и полупроводниковых нанокристаллов» УФН 176 23–57 (2006); DOI: 10.3367/UFNr.0176.200601b.0023

References (113) ↓ Cited by (21)

  1. Dagenais M, Mandel L Phys. Rev. A 18 2217 (1978)
  2. Nagourney W, Sandberg J, Dehmelt H Phys. Rev. Lett. 56 2797 (1986)
  3. Cook R J, Kimble H J Phys. Rev. Lett. 54 1023 (1985)
  4. Plenio M B, Knight P L Rev. Mod. Phys. 70 101 (1998)
  5. Moerner W E, Kador L Phys. Rev. Lett. 62 2535 (1989)
  6. Orrit M, Bernard J Phys. Rev. Lett. 65 2716 (1990)
  7. Moerner W E, Basche Th Angew. Chem. 32 457 (1993)
  8. Basché Th et al. (Eds) Single Molecule Optical Detection, Imaging And Spectroscopy (Munich: Wiley-VCH, 1997)
  9. Moerner W E, Orrit M Science 283 1670 (1999)
  10. Osad’ko I S Optika Spektrosk. 89 749 (2000)
  11. Osad’ko I S Selektivnaya Spektroskopiya Odinochnykh Molekul (M.: Fizmatlit, 2000); Osad’ko I S Selective Spectroscopy Of Single Molecules (Berlin: Springer, 2002)
  12. van den Bout D A et al. Science 277 1074 (1997)
  13. Ha T et al. Chem. Phys. Lett. 271 1 (1997)
  14. Lu H P, Xie X S Nature 385 143 (1997)
  15. Dickson R M et al. Nature 388 355 (1997)
  16. Lu H P, Xun L, Xie X S Science 282 1877 (1998)
  17. Hu D, Yu J, Barbara P F J. Am. Chem. Soc. 121 6936 (1999)
  18. van Oijen A M et al. Science 285 400 (1999)
  19. Gensch T et al. Angew. Chem. Int. Ed. 38 3752 (1999)
  20. Weiss S Science 283 1676 (1999)
  21. Yu J, Hu D, Barbara P F Science 289 1327 (2000)
  22. Hofkens J et al. J. Am. Chem. Soc. 122 9278 (2000)
  23. Nirmal M et al. Nature 383 802 (1996)
  24. Gammon D et al. Science 273 87 (1996)
  25. Efros Al L et al. Phys. Rev. B 54 4843 (1996)
  26. Pistol M-E et al. Phys. Rev. B 59 10725 (1999)
  27. Banin U et al. J. Chem. Phys. 110 1195 (1999)
  28. Kuno M et al. J. Chem. Phys. 112 3117 (2000)
  29. Kuno M et al. J. Chem. Phys. 115 1028 (2001)
  30. Sugisaki M et al. Phys. Status Solidi B 224 67 (2001)
  31. Shimizu K T et al. Phys. Rev. B 63 205316 (2001)
  32. Sugisaki M et al. Jpn. J. Appl. Phys. 41 958 (2002)
  33. Shimizu K T et al. Phys. Rev. Lett. 89 117401 (2002)
  34. Verberk R, van Oijen A M, Orrit M Phys. Rev. B 66 233202 (2002)
  35. Ambrose W P, Basché Th , Moerner W E J. Chem. Phys. 95 7150 (1991)
  36. Moerner W E et al. J. Phys. Chem. 98 7382 (1994)
  37. Anderson P W, Halperin B I, Varma C Philos. Mag. 25 1 (1972)
  38. Phillips W A J. Low Temp. 13 351 (1972)
  39. Boiron A-M et al. Chem. Phys. 247 119 (1999)
  40. Vainer Yu G i dr. Optika Spektrosk. 94 926 (2003)
  41. Mandel’ L, Vol’f E Opticheskaya Kogerentnost’ i Kvantovaya Optika (M.: Fizmatlit, 2000)
  42. Mandel L Opt. Lett. 4 205 (1979)
  43. Mandel L Proc. Phys. Soc. London 72 1037 (1958)
  44. Kelley P L, Kleiner W H Phys. Rev. 136 A316 (1964)
  45. Kim M S, Knight P L Phys. Rev. A 36 5265 (1987)
  46. Barkai E, Jung Y J, Silbey R Phys. Rev. Lett. 87 207403 (2001)
  47. Jung Y, Barkai E, Silbey R J Adv. Chem. Phys. 123 199 (2002)
  48. Kim M S, Knight P L, Wodkiewicz K Opt. Commun. 62 385 (1987)
  49. Osad’ko I S Zh. Eksp. Teor. Fiz. 113 1606 (1998)
  50. Basché Th et al. Phys. Rev. Lett. 69 1516 (1992)
  51. Mollow B R Phys. Rev. A 12 1919 (1975)
  52. Osad’ko I S Zh. Eksp. Teor. Fiz. 98 1045 (1990)
  53. Zheng Y, Brown F L H Phys. Rev. Lett. 90 238305 (2003)
  54. Zheng Y, Brown F L H J. Chem. Phys. 119 11814 (2003)
  55. Osad’ko I S Zh. Eksp. Teor. Fiz. 128 77 (2005)
  56. Short R, Mandel L Phys. Rev. Lett. 51 384 (1983)
  57. Osad’ko I S, Yershova L B J. Lumin. 86 211 (2000)
  58. Verberk R, Orrit M J. Chem. Phys. 119 2214 (2003)
  59. Zaitsev N N, Osad’ko I S Zh. Eksp. Teor. Fiz. 104 4042 (1993)
  60. Donskoi D V, Zaitsev N N, Osad’ko I S Chem. Phys. 176 135 (1993)
  61. Osad’ko I S Zh. Eksp. Teor. Fiz. 109 805 (1996)
  62. Osad’ko I S Zh. Eksp. Teor. Fiz. 116 962 (1999)
  63. Osad’ko I S, Yershova L B J. Chem. Phys. 112 9645 (2000)
  64. Osad’ko I S, Yershova L B J. Lumin. 87 - 89 184 (2000)
  65. Kilin S Ya et al. Phys. Rev. A 57 1400 (1998)
  66. Dalibard J, Castin Y, Mølmer K Phys. Rev. Lett. 68 580 (1992)
  67. Geva E, Skinner J L J. Phys. Chem. B 101 8920 (1997)
  68. Geva E, Skinner J L J. Chem. Phys. 109 4920 (1998)
  69. Plakhotnik T J. Lumin. 83 - 84 221 (1999)
  70. Makarov D E, Metiu H J. Chem. Phys. 115 5989 (2001)
  71. Dum R, Zoller P, Ritsch H Phys. Rev. A 45 4879 (1992)
  72. Wang J, Wolynes P J. Chem. Phys. 110 4812 (1999)
  73. Cao J Chem. Phys. Lett. 327 38 (2000)
  74. Gardiner C W, Parkins A S, Zoller P Phys. Rev. A 46 4363 (1992)
  75. Reynaud S Ann. Phys. (Paris) 8 315 (1983)
  76. Barsegov V, Chernyak V, Mukamel S J. Chem. Phys. 116 4240 (2002)
  77. Barkai E, Silbey R, Zumofen G Phys. Rev. Lett. 84 5339 (2000)
  78. Naumov A V et al. Phys. Rev. B 63 212302 (2001)
  79. Maier H et al. Phys. Rev. Lett. 74 5252 (1995)
  80. Osad’ko I S, Lobanov A N Optika Spektrosk. 99 306 (2005)
  81. Osad’ko I S In Spectroscopy And Excitation Dynamics Of Condensed Molecular Systems (Modern Problems in Condensed Mater Sciences, Vol. 4, Eds V M Agranovich, R M Hochstrasser) (Amsterdam: North-Holland, 1983)
  82. Osad’ko I S Phys. Rep. 206 43 (1991)
  83. Gladenkova S N, Osad’ko I S Chem. Phys. Lett. 187 628 (1991)
  84. Vainer Yu G et al. J. Chem. Phys. 116 8959 (2002)
  85. Anderson P W J. Phys. Soc. Jpn. 9 316 (1954)
  86. Klauder J R, Anderson P W Phys. Rev. 125 912 (1962)
  87. Reinecke T L Solid State Commun. 32 1103 (1979)
  88. Bai Y S, Fayer M D Phys. Rev. B 39 11066 (1989)
  89. Reilly P D, Skinner J L J. Chem. Phys. 101 959 (1994); Reilly P D, Skinner J L J. Chem. Phys. 101 965 (1994)
  90. Osad’ko I S, Khots E V Single Mol. 3 236 (2002)
  91. Osad’ko I S, Khots E V Optika Spektrosk. 94 949 (2003)
  92. Osad’ko I S Zh. Eksp. Teor. Fiz. 120 991 (2001)
  93. Osad’ko I S, Yershova L B J. Chem. Phys. 111 7652 (1999)
  94. Zilker S J, Haarer D Chem. Phys. 220 167 (1997)
  95. Hannig G et al. Mol. Cryst. Liq. Cryst. 291 11 (1996)
  96. Tchenio P, Myers A B, Moerner W E J. Lumin. 56 1 (1993)
  97. Fleury L et al. J. Lumin. 56 15 (1993)
  98. Kozankiewicz B, Bernard J, Orrit M J. Chem. Phys. 101 9377 (1994)
  99. Naumov A V et al. J. Chem. Phys. 116 8132 (2002)
  100. Vainer Yu G i dr. Optika Spektrosk. 94 936 (2003)
  101. Vainer Yu G et al. J. Lumin. 107 287 (2004)
  102. Mirzov O et al. Chem. Phys. Lett. 386 286 (2004)
  103. Osad’ko I S Zh. Eksp. Teor. Fiz. 123 696 (2003)
  104. Harrison N T et al. Phys. Rev. B 53 15815 (1996)
  105. Swager T M, Gil C J, Wrighton M S J. Phys. Chem. 99 4886 (1995)
  106. Osad’ko I S, Chigirev A R Fiz. Tverd. Tela 23 538 (1981)
  107. Efros Al L, Rosen M Phys. Rev. Lett. 78 1110 (1997)
  108. Cichos F, Martin J, von Borczyskowski C Phys. Rev. B 70 115314 (2004)
  109. Cichos F, Martin J, von Borczyskowski C J. Lumin. 107 160 (2004)
  110. Osad’ko I S Pis’ma ZhETF 79 522 (2004)
  111. Osad’ko I S Chem. Phys. 316 99 (2005)
  112. Krauss T D, Brus L E Phys. Rev. Lett. 83 4840 (1999)
  113. Krauss T D, O’Brien S, Brus L E J. Phys. Chem. B 105 1725 (2001)
© 1918–2024 Uspekhi Fizicheskikh Nauk
Email: ufn@ufn.ru Editorial office contacts About the journal Terms and conditions